Towards a spray-coating method for the detection of low-dose compounds in pharmaceutical tablets using surface-enhanced Raman chemical imaging (SER-CI)

Cailletaud, Johan; De Bleye, Charlotte; Dumont, Elodie; Sacre, Pierre-Yves; Gut, Yoann; Bultel, Laurent; Ginot, Yves-Michel; Hubert, Philippe; Ziemons, Eric

doi:10.1016/j.talanta.2018.06.037

Article (Scientific journals)

Towards a spray-coating method for the detection of low-dose compounds in pharmaceutical tablets using surface-enhanced Raman chemical imaging (SER-CI)

Cailletaud, Johan; De Bleye, Charlotte; Dumont, Elodie et al.

2018 • In Talanta, 188, p. 584-592

Peer Reviewed verified by ORBi

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https://hdl.handle.net/2268/225319

DOI
10.1016/j.talanta.2018.06.037

PubMed
30029417

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Keywords :

Surface-enhanced Raman scattering (SERS); Spray-coating; Metallic colloidal suspension; Silver nanoparticles; Chemical imaging; Pharmaceutical tablets

Abstract :

[en] Surface-enhanced Raman chemical imaging (SER-CI) is a highly sensitive analytical tool recently used in the pharmaceutical field owing to the possibility to obtain high sensitivity along with spatial information. However, the covering method of the pharmaceutical samples such as tablets with metallic nanoparticles is a major issue for SER-CI analyses due to the difficulty to obtain a homogeneous covering of tablet surface with the SERS substrates. In this context, a spray-coating method was proposed in order to fully exploit the potential of SER-CI. A homemade apparatus has been developed from an electrospray ionization (ESI) probe in order to cover the pharmaceutical tablets with the colloidal suspension in a homogeneous way. The silver substrate was pulled through the airbrush by a syringe pump which was then nebulized into small droplets due to the contact of the solution with the gas flow turbulence. A robust optimization of the process was carried out by adjusting experimental parameters such as the liquid flow rate and the spraying time. Besides, the performances of this spraying technique were compared with two others covering methods found in the literature which are drop casting and absorption coating. A homogeneity study, conducted by SER-CI and matrix assisted laser desorption/ ionization mass spectrometry imaging (MALDI-MSI) applied to the different covering techniques was performed. The influence of the metallic nanoparticles deposit on soluble compounds was also investigated in order to highlight the advantages of using this new spray coating approach.

Research Center/Unit :

CIRM - Centre Interdisciplinaire de Recherche sur le Médicament - ULiège

Disciplines :

Pharmacy, pharmacology & toxicology

Author, co-author :

Cailletaud, Johan ; Université de Liège - ULiège > Département de pharmacie > Chimie analytique

De Bleye, Charlotte ; Université de Liège - ULiège > Département de pharmacie > Département de pharmacie

Dumont, Elodie ; Université de Liège - ULiège > Département de pharmacie > Chimie analytique

Sacre, Pierre-Yves ; Université de Liège - ULiège > Département de pharmacie > Chimie analytique

Gut, Yoann; Technologie Servier

Bultel, Laurent; Technologie Servier

Ginot, Yves-Michel

Hubert, Philippe ; Université de Liège - ULiège > Département de pharmacie > Chimie analytique

Ziemons, Eric ; Université de Liège - ULiège > Département de pharmacie > Département de pharmacie

Language :

English

Title :

Towards a spray-coating method for the detection of low-dose compounds in pharmaceutical tablets using surface-enhanced Raman chemical imaging (SER-CI)

Publication date :

01 October 2018

Journal title :

Talanta

ISSN :

0039-9140

eISSN :

1873-3573

Publisher :

Elsevier, Netherlands

Volume :

188

Pages :

584-592

Peer reviewed :

Peer Reviewed verified by ORBi

Available on ORBi :

since 15 June 2018

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