Unusual thermoelectric behavior of packed crystalline granular metals

Ausloos, Marcel; Pekala, Marek; Latuch, J.; Mucha, Jan; Vanderbemden, Philippe; Vertruyen, Bénédicte; Cloots, Rudi

doi:10.1063/1.1808248

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Unusual thermoelectric behavior of packed crystalline granular metals

Ausloos, Marcel; Pekala, Marek; Latuch, J. et al.

2004 • In Journal of Applied Physics, 96 (12), p. 7338-7345

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https://hdl.handle.net/2268/1746

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10.1063/1.1808248

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Keywords :

thermoelectric power; granular metals; electrical resistivity

Abstract :

[en] Loosely packed granular materials are intensively studied nowadays. Electrical and thermal transport properties should reflect the granular structure, as well as intrinsic properties. We have compacted crystalline CaAl-based metallic grains and studied the electrical resistivity and the thermoelectric power as a function of temperature (T) from 15 to 300 K. Both properties show three regimes as a function of temperature. It should be pointed out: (i) The electrical resistivity continuously decreases between 15 and 235 K, (ii) with various dependencies, e.g., similar ~ T(-3/4) at low T, while (iii) the thermoelectric power (TEP) is positive, (iv) shows a bump near 60 K, and (v) presents a rather unusual square root of temperature dependence at low temperature. It is argued that these three regimes indicate a competition between geometric and thermal processes-for which a theory seems to be missing in the case of TEP. The microchemical analysis results are also reported, indicating a complex microstructure inherent to the phase diagram peritectic intricacies of this binary alloy. (C) 2004 American Institute of Physics.

Research Center/Unit :

SUPRATECS - Services Universitaires pour la Recherche et les Applications Technologiques de Matériaux Électro-Céramiques, Composites, Supraconducteurs - ULiège

Disciplines :

Physics

Author, co-author :

Ausloos, Marcel ; Université de Liège - ULiège > Département de physique > Physique statistique appliquée et des matériaux

Pekala, Marek; University of Warsaw

Latuch, J.; University of Warsaw

Mucha, Jan ; Institute of Low Temperature and Structure Research, Wroclaw

Vanderbemden, Philippe ; Université de Liège - ULiège > Capteurs et systèmes de mesures électriques

Vertruyen, Bénédicte ; Université de Liège - ULiège > Chimie inorganique structurale

Cloots, Rudi ; Université de Liège - ULiège > Chimie inorganique structurale

Language :

English

Title :

Unusual thermoelectric behavior of packed crystalline granular metals

Publication date :

December 2004

Journal title :

Journal of Applied Physics

ISSN :

0021-8979

eISSN :

1089-7550

Publisher :

Amer Inst Physics, Melville, United States - New York

Volume :

Issue :

Pages :

7338-7345

Peer reviewed :

Peer Reviewed verified by ORBi

Additional URL :

http://link.aip.org/link/?JAPIAU/96/7338/1

Funders :

Polish Committee for Scientific Research (KBN)

Commentary :

Copyright (2004) American Institute of Physics. This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics. The following article appeared in J. Appl. Phys. 96, 7338 (2004) and may be found at http://link.aip.org/link/?JAPIAU/96/7338/1.

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