Steering Quantum Dynamics through Electronic Entanglement in Molecules Pumped by Atto and Few Femto Second Pulses

Chemical lasers; Chemical reactions; Dynamics; Electro-optical waveguides; Force; Laser excitation; Lasers and electrooptics; Pump lasers; Quantum entanglement; Ultrafast electronics; Electro-optical; Electro-optical waveguide; Electronic entanglement; Femtoseconds; Laser and electrooptic; Pump laser; Quantum dynamics; Ultra-fast; Ultrafast electronic; Process Chemistry and Technology; Computer Networks and Communications; Civil and Structural Engineering; Electrical and Electronic Engineering; Electronic, Optical and Magnetic Materials; Instrumentation; Atomic and Molecular Physics, and Optics

Abstract :

[en] Broad energy band width atto pulses excite superposition of electronic states that entangle electronic and nuclear motions. We discuss how to exploit this entanglement to steer the force on the nuclei and control chemical reactivity.

Disciplines :

Chemistry

Author, co-author :

Remacle, Françoise ; Université de Liège - ULiège > Département de chimie (sciences) > Laboratoire de chimie physique théorique

Language :

English

Title :

Steering Quantum Dynamics through Electronic Entanglement in Molecules Pumped by Atto and Few Femto Second Pulses

Publication date :

2024

Event name :

CLEO 2024

Event organizer :

APS

Event place :

Charlotte, Usa

Event date :

07-05-2024 => 10-05-2024

By request :

Yes

Audience :

International

Main work title :

2024 Conference on Lasers and Electro-Optics, CLEO 2024

Publisher :

Institute of Electrical and Electronics Engineers Inc.

ISBN/EAN :

978-1-957171-39-5

Peer review/Selection committee :

Peer reviewed

Additional URL :

https://opg.optica.org/viewmedia.cfm?URI=CLEO_FS-2024-FM2B.4&seq=0

Funders :

American Elements
IEEE - Institute of Electrical and Electronics Engineers

Available on ORBi :

since 03 July 2025

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Bibliography

F. Remacle and R. D. Levine, Proc. Natl. Acad. Sci. USA 103 (18), 6793-6798 (2006)
F. Remacle, et al., Phys. Rev. Lett. 99 (18), 183902 (2007)
B. Mignolet, et al., J. Phys. B: At. Mol. Opt. Phys. 47 (12), 124011 (2014).
Manual Cardosa-Gutierrez, R. D. Levine, F. Remacle, ChemRxiv, DOI: 10.26434/chemrxiv-2023-bqnt6, (2023).
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M. Blavier, et al., Chem. Phys. Lett. 804, 139885 (2022).
M. Cardosa-Gutierrez, R. D. Levine, F. Remacle, 2023, submitted.
A. Valentini, et al., Phys. Chem. Chem. Phys. 22 (39), 22302-22313 (2020).
C.E.M. Gonçalves, R.D. Levine, F. Remacle, Phys. Chem. Chem. Phys. 23 (2021) 12051-12059
M. Blavier, et al., J. Phys. Chem. A 125 (43), 9495-9507 (2021).