Raw wastewater; Sandy soil; Long-term; Invariant element; Pedo-geochemical background
Abstract :
[en] Trace metal inputs reconstitution and migration assessment in a sandy Luvisol after 100 years of massive irrigation with raw wastewaters. Raw wastewaters were massively spread on sandy luvisols near Paris from 1899 to 2002, leading to high trace metals (TM) pollution of soils. Mass balance calculations were performed on a soil profile to assess vertical migration of TM. The contamination was estimated by subtracting the natural pedo-geochemical background of the horizons. TM inputs were estimated using Cr as an invariant. It is shown that Pb and Cr remained in the surface horizon, while Ni, Cd, Cu and Zn migrated downward, being more or less trapped depending on the physicochemical properties of the horizons.
Disciplines :
Physical, chemical, mathematical & earth Sciences: Multidisciplinary, general & others
Ahumada I., Mendoza J., Navarrete E., and Ascar L. Sequential extraction of heavy metals in soils irrigated with wastewater. Commun. Soil Sci. Plant Anal. 30 9-10 (1999) 1507-1519
Alloway B.J. Cadmium. In: Alloway B.J. (Ed). Heavy Metals in Soils (1990), Blackie, Glasgow 100-124
Alloway B.J. Heavy Metals in Soils (1990), Blackie, Glasgow, Royaume-Uni
B.J. Alloway, The mobilisation of trace elements in soils, in: R. Prost (Ed.), Contaminated Soils, in: Les colloques no 85, Actes du 3e ICOBTE, Inra, Paris, 15-19 mai 1995
Baize D. Recherche des contaminations par démarche typologique. Teneurs totales en éléments traces métalliques dans les sols (France) (1997), Inra, Paris 215-218
Baize D. Guide des analyses en pédologie (2000), Inra, Paris
Bataillard P., Cambier P., and Picot C. Short-term transformations of lead and cadmium compounds in soil after contamination. Eur. J. Soil Sci. 54 2 (2003) 365-376
Boyle M., and Fuller W.H. Effect of municipal solid waste leachate composition on zinc migration through soils. J. Environ. Qual. 16 4 (1987) 357-360
Bruand A. Toward conditions favourable to mobility of trace elements in soils. C. R. Geoscience 337 (2005) 549-550
Camobreco V., Richards B.K., Steenhuis T.S., Peverly J.H., and McBride M.B. Movement of heavy metals through undisturbed and homogenized soil columns. Soil Sci. 161 11 (1996) 740-750
L. Citeau, Étude des colloïdes naturels présents dans les eaux gravitaires de sols contaminés : relation entre nature des colloïdes et réactivité vis-à-vis des métaux (Zn, Cd, Pb, Cu), thèse, INA-PG, Paris, 2004 (251 p.)
Cornu S., Neal C., Ambrosi J.P., Whitehead P., Neal M., Sigolo J., et al. The environmental impact of heavy metals from sewage sludge in ferrasols (Sao Paulo, Brazil). Sci. Total Environ. 271 (2001) 27-48
Dagnelie P. Statistique théorique et appliquée, tome 2 (1998), De Boeck & Larcier, Bruxelles
Domergue F.L., and Vedy J.-C. Mobility of heavy metals in soil profiles. Int. J. Environ. Anal. Chem. 46 (1992) 13-23
Emmerich W.E., Lund L.J., Page A.L., and Chang A.C. Movement of heavy metals in sewage sludge-treated soils. J. Environ. Qual. 11 2 (1982) 174-178
Emmerich W.E., Lund L.J., Page A.L., and Chang A.C. Predicted solution phase forms of heavy metals in sewage sludge-treated soils. J. Environ. Qual. 11 2 (1982) 182-186
Haiyan W., and Stuanes A.O. Heavy metal pollution in air-water-soil-plant system of Zhuzhou City, Hunan Province, China. Water Air Soil Pollut. 147 1-4 (2003) 79-107
Jiries A.G., Al-Nasir F.M., and Beese F. Pesticide and heavy metals residue in wastewater, soil and plants in wastewater disposal site near Al-Lajoun Valley, Karak/Jordan. Water Air Soil Pollut. 133 1-4 (2002) 97-104
Kabata-Pendias A. Behavioural properties of trace metals in soils. Appl. Geochem. 2 Suppl. (1993) 3-9
Kiekens L. Zinc. In: Alloway B.J. (Ed). Heavy Metals in Soils (1990), Blackie, Glasgow 261-279
Lamy I., Bourgeois S., and Bermond A. Soil cadmium mobility as a consequence of sewage sludge disposal. J. Environ. Qual. 22 4 (1993) 731-737
Lamy I., van Oort F., Dère C., and Baize D. Use of major- and trace-element correlations to assess metal migration in sandy luvisols irrigated with wastewater. Eur. J. Soil Sci. (2006) 10.1111/j.1365-2389.2005.00765.x
Legret M., Divet L., and Juste C. Migration et spéciation des métaux lourds dans un sol soumis à des épandages de boues de station d'épuration à très forte charge en Cd et Ni. Water Res. 22 8 (1988) 953-959
Lozet J., and Mathieu C. Dictionnaire de science du sol (1990), Lavoisier, Paris
Luo Y., Jiang X., Wu L., Song J., Wu S., Lu R., et al. Accumulation and chemical fractionation of Cu in a paddy soil irrigated with Cu-rich wastewater. Geoderma 115 1-2 (2003) 113-120
McBride M.B. Environmental Chemistry of Soils (1994), Oxford University Press, New York
McBride M.B., Richards B., Steenhuis T., Russo J., and Sauvé S. Mobility and solubility of toxic metals and nutrients in soil fifteen years after sludge application. Soil Sci. 162 7 (1997) 487-500
McGrath S.P. Long-term studies of metal transfers following application of sewage sludge. Pollut. Transp. Fate Ecosyst. 6 Suppl. (1987) 301-317
McGrath S.P., and Lane P.W. An explanation for the apparent losses of metals in a long-term field experiment with sewage sludge. Environ. Pollut. 60 (1989) 235-256
Mehra O.P., and Jackson M.L. Iron oxide removal from soils and clay by a dithionite-citrate system buffered with sodium bicarbonate. Clays Clay Miner. 7 (1960) 317-327
Quantin C., Becquer T., and Berthelin J. Mn-oxide: a major source of easily mobilisable Co and Ni under reducing conditions in New Caledonia Ferralsols. C. R. Geoscience 334 4 (2002) 273-278
Richards B., Steenhuis T., Peverly J., and McBride M. Metal mobility at an old, heavily loaded sludge application site. Environ. Pollut. 99 (1998) 965-977
Romkens P.F., Bril J., and Salomons W. Interaction between Ca2+ and dissolved organic carbon: implications for metal mobilization. Appl. Geochem. 11 1/2 (1996) 109-115
Sager M. Chemical speciation and environmental mobility of heavy metals in sediments and soils. In: Stoeppler M. (Ed). Hazardous Metals in the Environment (1992), Elsevier, Amsterdam 133-175
Schirado T., Vergara I., Schalscha B., and Pratt P. Evidence of movement of heavy metals in a soil irrigated with untreated wastewater. J. Environ. Qual. 15 1 (1986) 9-12
Simpson S.L., Maher E.J., and Jolley D.F. Processes controlling metal transport and retention as metal-contaminated groundwaters efflux through estuarine sediments. Chemosphere 56 9 (2004) 821-831
Temminghoff E.J., van der Zee S.E., and de Haan F.A. Effects of dissolved organic matter on the mobility of copper in a contaminated sandy soil. Eur. J. Soil Sci. 49 4 (1998) 617-628
Tomassone R., Lesquoy E., and Millier C. La régression : nouveaux regards sur une ancienne méthode statistique (1983), Inra, Paris
Yadav R.K., Goyal B., Sharma R.K., Dubey S.K., and Minhas P.S. Post-irrigation impact of domestic sewage effluent on composition of soils, crops and ground water - a case study. Environ. Int. 28 6 (2002) 482-486
Yingming L., and Corey R.B. Redistribution of sludge-borne cadmium, copper, and zinc in a cultivated plot. J. Environ. Qual. 22 1 (1993) 1-8
