Abstract :
[en] Our quantum device is a solid-state array of semiconducting quantum dots
that is addressed and read by 2D electronic spectroscopy. The experimental ultrafast
dynamics of the device is well simulated by solving the time-dependent Schrödinger equation
for a Hamiltonian that describes the lower electronically excited states of the dots and three
laser pulses. The time evolution induced in the electronic states of the quantum device is
used to emulate the quite different nonequilibrium vibrational dynamics of a linear triatomic
molecule. We simulate the energy transfer between the two local oscillators and, in a more
elaborate application, the expectation values of the quantum mechanical creation and
annihilation operators of each local oscillator. The simulation uses the electronic coherences
engineered in the device upon interaction with a specific sequence of ultrafast pulses. The
algorithm uses the algebraic description of the dynamics of the physical problem and of the hardware.
Disciplines :
Physical, chemical, mathematical & earth Sciences: Multidisciplinary, general & others
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