Precision measurement of radioactivity in Gamma-rays spectrometry using two HPGe detectors (BEGe-6530 and GC0818-7600SL models) comparison techniques: Application to the soil measurement.
[en] To obtain high quality of results in gamma spectrometry, it is necessary to select the best HPGe detector for particular measurements, to calibrate energy and efficiency of gamma detector as accurate as possible. To achieve this aim, the convenient detector model and gamma source can be very useful. The purpose of this study was to evaluate the soil specific activity using two HPGe model (BEGe-6530 and GC0818-7600SL) by comparing the results of the two detectors and the technics used according to the detector type. The relative uncertainty activity concentration was calculated for 226Ra, 232Th and 40K. For broad energy germanium detector, BEGe-6530, the relative uncertainty concentration ranged from 2.85 to 3.09% with a mean of 2.99% for 226Ra, from 2.29 to 2.49% with a means of 2.36% for 232Th and from 3.47 to 22.37% with a mean of 12.52% for 40K. For GC0818-7600SL detector, it was ranged from 10.45 to 25.55% with a mean of 17.10% for 226Ra, from 2.54 to 3.56% with a means of 3.10% for 232Th and from 3.42 to 7.65% with a mean of 5.58% for 40K. The average report between GC0818-7600SL model and BEGe-6530 model was calculated and showed the mean value of 3.36. The main study was based on the following points:
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Determination of The relative uncertainty activity concentration of 226Ra, 232Th and 40K
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Determination of the relative uncertainty related to the radium equivalent activity to compare the performance of the two detection systems
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Proved that the activity concentration determination in gamma spectrometry depended on the energy range emitted by a radionuclide.
This study showed that the standard deviation measurement was less important to the result realized with BEGe-6530 HPGe model. Our findings were demonstrated that the results of the Broad Energy Germanium detector were more reliable.
Research Center/Unit :
Spectroscopie Atomique et Nucleaire, Archeometrie ULG
Samafou Penabei; Centre for Atomic Molecular Physics and Quantum Optics, University of Douala, P.O. Box 8580, Douala-Cameroon
NDONTCHUENG MOYO, Maurice; Department of Physics, Faculty of Science, University of Douala, P.O. Box 24157, Douala, Cameroon > National Radiation Protection Agency, P.O. Box 33732, Yaounde, Cameroon
Chene, Grégoire ; Université de Liège > Centre européen en archéométrie
NGUELEM MEKONTSO, Eric Jilbert; Department of Physics, Faculty of Science, University of Douala, P.O. Box 24157, Douala, Cameroon > National Radiation Protection Agency, P.O. Box 33732, Yaounde, Cameroon
NGWA EBONGUE, Alexandre; Centre for Atomic Molecular Physics and Quantum Optics, University of Douala, P.O. Box 8580, Douala-Cameroon
MOTAPON, Ousmanou; Department of Physics, Faculty of Science, University of Douala, P.O. Box 24157, Douala, Cameroon
Strivay, David ; Université de Liège > Département de physique > Spectroscopie atomique et nucléaire, archéométrie
Language :
English
Title :
Precision measurement of radioactivity in Gamma-rays spectrometry using two HPGe detectors (BEGe-6530 and GC0818-7600SL models) comparison techniques: Application to the soil measurement.
Orabi, H., Al-Shareaif, A., El Galefi, M., Gamma-ray measurements of naturally occurring radioactive sample from Alkharje City (2006) J. Rad. Nucl. Chem., 269, pp. 99-102
United Nations Scientific Committee on the Effect of Atomic Radiation, Report to the General Assembly. Annex B: Exposures from Natural Radiation Sources (2000)
Knoll Glenn, F., Radiation Detection and Measurement (1989), second ed. John Wiley & Sons. Inc New York
Ndontchueng, M.M., Nguelem, E.J.M., Njinga, R.L., Simo, A., Guembou, J.C.S., Gamma emitting radionuclides in soils from selected areas in Douala-Bassa zone littoral region of Cameroon (2014) ISRN Spectroscopy, p. 8. , (Article ID 245125)
Morera-Gómez, Y., Cartas-Aguila, H.A., Alonso-Hernández, C.M., Nuñez-Duartes, C., Validation of an efficiency calibration procedure for a coaxial n-type and a well-type HPGe detector used for the measurement of environmental radioactivity (2016) Nucl. Inst. Meth. in Phys. Res. Sect. A, 818 (11), pp. 51-56
Tzortzis, M., Svoukis, E., Tsetos, H., A comprehensive study of natural gamma radioactivity levels and associated dose rates from surface soils in Cyprus (2004) Rad. Prot. Dos., 109 (3), pp. 217-224
Britton, R., Davies, A.V., Burnett, J.L., Jackson, M.J., A high-efficiency HPGe coincidence system for environmental analysis (2015) J. Env. Rad., 146, pp. 1-5
Ababneh, A.M., Eyadeh, M.M., Coincidence summing corrections in HPGe gamma-ray spectrometry for Marinelli-beakers geometry using peak to total (P/T) calibration (2015) J. Rad. Res. Appl. Sci., pp. 323-327
Ndontchueng, M.M., Nguelem, E.J.M., Motapon, O., Njinga, R.L., Simo, A., Guembou, J.C.S., Yimele, B., Radiological hazards in soil from the bauxite deposits sites in dschang region of Cameroon (2015) Brit. J. Appl. Sci. Tech., 5 (4), pp. 342-352
Venkataraman, R., Bronson, F., Abashkevich, V., Young, B.M., Field, M., Validation of in situ object counting system (ISOCS) mathematical efficiency calibration software (1999) Nucl. Instrum. Methods Phys. Res. Sect. A: Accelerat. Spectrom. Detect. Assoc. Equip., 422, pp. 450-454
Hult, M., Lutter, G., Yüksel, A., Marissens, G., Misiaszek, M., Rosengård, U., Comparison of background in underground HPGe-detectors in different lead shield configurations (2013) Appl. Radi. Isot., 81, pp. 103-108
Slaninka, A., Slávik, O., Necas, V., Uncertainty analysis of in-situ gamma spectrometry measurements of air cleaning filter cartridges and 200L drums by a HPGe detector (2010) Appl. Radiat. Isot., 68, pp. 1273-1277
Beretka, J., Mathew, P.J., Natural radioactivity of Australian build-ing materials, industrial wastes and by-products (1985) Health Phys., 48, pp. 87-95
Keyser, R., Twomey, T., Wagner, S., Benefits of using super-Large germanium gamma-Ray detectors for the quantitative determination of environmental radionuclides (1990) Radioact. Radiochem., 1 (2), pp. 46-56
ORTEC, Modular Pulse Processing Electronics Catalog (2001), pp. 83-84. , www.ortec-online.com, Oak Ridge USA
ORTEC, www.ortec-online.com, The Best Choice of High Purity Germanium (HPGe) Detector, available from
Yavar, A., Sarmani, S.B., Khoo, K.S., The better efficiency calibration for HPGe detector by comparing the single point gamma sources and multi-nuclides gamma sources for k0-NAA method (2014) IOSR J. Appl. Phys., 6 (3), pp. 54-56. , (ISSN: 2278–4861)
Gervino, G., Mana, G., Palmisano, C., Optimization of statistical methods for HpGe gamma-ray spectrometer used in wide count rate ranges (2015) Nuc. Inst. Meth. Phys. Res. Sect. A Vol, 824, pp. 99-100
Sajo-Bohus, L., Rosso, D., Sajo, A.M., Castelli Napoli, D.R., Fioretto, E., Menegazzo, R., Barros, H., Liendo, J., HPGe detectors long time behaviour in high-resolution γ spectrometry (2011) Nucl. Inst. Meth. Phys. Res. Sect. A, 648 (1), pp. 132-138
Crespi, F.C.L., Camera, F., Million, B., Sassi, M., Wieland, O., Bracco, A., A novel technique for the characterization of a HPGe detector response based on pulse shape comparison (2008) Nucl. Inst. Meth. Phys. Res. Sect. A Vol., 593, pp. 440-447
Jenkins, R., Gould, R.W., Gedcke, D., (1981) Quantitative X-Ray Spectrometry, 209-229. , first ed. Marcel Dekker New York
Gedcke, D.A., ORTEC Application Note AN57, Dealing with Dead Time Distortion in a Time Digitizer (2001)
Gedcke, D.A., ORTEC Application Note AN58, How Histogramming and Counting Statistics Affect Peak Position Precision (2001)
Gedcke, D.A., ORTEC How Counting Statistics Controls Detection Limits and Peak Precision (2009)
CANBERRA Manual, Nuclear Measurement Solutions for Safety, Security and the Environment, Broad Energy Germanium Detectors (BEGe) C40426-11/13 (2013), http://www.canberra.com/products/detectors/pdf/BEGe-SS-C40426.pdf