NHC-Ru complexes-  Friendly catalytic tools for manifold chemical transformations

[en] N-Heterocyclic carbenes are now commonly encountered in organometallic and inorganic coordination chemistry. The increasing attention they enjoy is due to their ability to act as ancillary ligands in a growing number of transition metal catalysts or even to play the role of nucleophilic reagents and catalysts in diverse organic transformations. As a fine addition to the NHC-Ru-alkylidenes, popular for their tremendous success in metathesis chemistry, an array of robust and stable Ru-NHCs has proven their utility in non-metathetical reactions. The present review surveys different classes of Ru-NHCs and their applications as efficient catalysts (or precatalysts) in several types of fundamental organic processes e.g. hydrogenation, hydrogen transfer, isomerization, cycloisomerization, cyclopropanation, hydrosilylation, allylation and deallylation, enol-ester synthesis, heterocycle synthesis, C-C alkyne coupling, Kharasch addition and ATRP. A special section is devoted to tandem processes some of which include concurrent or sequential metathesis steps. Relevant mechanistic and stereochemical aspects related to NHC-Ru catalysis will be highlighted. (c) 2006 Elsevier B.V. All rights reserved.

Disciplines :

Chemistry

Author, co-author :

Dragutan, Valerian

Dragutan, Ileana

Delaude, Lionel ; Université de Liège - ULiège > Chimie macromoléculaire et catalyse organique

Demonceau, Albert ; Université de Liège - ULiège > Chimie macromoléculaire et catalyse organique

Language :

English

Title :

NHC-Ru complexes- Friendly catalytic tools for manifold chemical transformations

Publication date :

2007

Journal title :

Coordination Chemistry Reviews

ISSN :

0010-8545

Publisher :

Elsevier Science, Lausanne, Switzerland

Volume :

251

Issue :

5-6

Pages :

765-794

Peer reviewed :

Peer Reviewed verified by ORBi

Available on ORBi :

since 26 June 2009

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