3D printing; Ion conduction; Polymer electrolytes; Room temperature ionic liquids; Stereolithography; 3-D printing; 3D-printing; Alkylammonium cations; Ionogels; Mesylates; Polymer electrolyte; Protic ionic liquids; Triflates; Atomic and Molecular Physics, and Optics; Physical and Theoretical Chemistry
Abstract :
[en] A range of protic ionic liquids (PILs) based on tri-n-alkylammonium cations and mesylate/triflate anions were incorporated into a polymer matrix to form ionogels (IGs). These systems were investigated for their thermal and electrochemical behaviour, as well as under the aspect of ion motion via PFG-NMR. The ionic conductivities of the ILs/IGs are in the range of 10-4-10-3 S/cm-1 at elevated temperatures and the diffusion coefficients are around 10-11 m2 s-1. Successful 3D printing of an IG with 70 wt % of IL is possible via stereolithography approaches, opening up applications in, e. g., structured ion-conductive membranes.
Disciplines :
Chemistry
Author, co-author :
Lange, Alyna; Institute of Chemistry, University of Potsdam, Karl-Liebknecht-Straße 24-25, 14476, Potsdam-Golm, Germany
Arwish, Sajal; Institute of Physical Chemistry, University of Münster, Corrensstraße 28/30, 48149, Münster, Germany
Rensonnet, Aurélie ; Université de Liège - ULiège > Molecular Systems (MolSys)
Elamin, Khalid; Department of Chemistry and Chemical Engineering, Applied Chemistry, Chalmers University of Technology, Gothenborg, 41296, Sweden
Abdurrokhman, Iqbaal; Department of Chemistry and Chemical Engineering, Applied Chemistry, Chalmers University of Technology, Gothenborg, 41296, Sweden
Wojnarowska, Zaneta; Institute of Physics, The University of Silesia in Katowice, 75 Pułku Piechoty 1 A, 41-500, Chorzow, Poland
Rosenwinkel, Mark; Institute of Physical Chemistry, University of Münster, Corrensstraße 28/30, 48149, Münster, Germany
Malherbe, Cédric ; Université de Liège - ULiège > Département de chimie (sciences) > Chimie analytique inorganique
Schönhoff, Monika; Institute of Physical Chemistry, University of Münster, Corrensstraße 28/30, 48149, Münster, Germany
Zehbe, Kerstin; Institute of Chemistry, University of Potsdam, Karl-Liebknecht-Straße 24-25, 14476, Potsdam-Golm, Germany
Taubert, Andreas ; Institute of Chemistry, University of Potsdam, Karl-Liebknecht-Straße 24-25, 14476, Potsdam-Golm, Germany
Language :
English
Title :
3D Printable Polymer Electrolytes for Ionic Conduction based on Protic Ionic Liquids.
Publication date :
10 November 2024
Journal title :
Chemphyschem: A European Journal of Chemical Physics and Physical Chemistry
ISSN :
1439-4235
eISSN :
1439-7641
Publisher :
John Wiley and Sons Inc, Germany
Pages :
e202400849
Peer reviewed :
Peer Reviewed verified by ORBi
Funders :
Universität Potsdam Energimyndigheten SSF - Stiftelsen för Strategisk Forskning
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