Optical Excitation of Coherent THz Dynamics of the Rare-Earth Lattice through Resonant Pumping of f-f Electronic Transition in a Complex Perovskite DyFeO3

Gareev, T. T.; Sasani, Alireza; Khusyainov, D. I.; Bousquet, Eric; Gareeva, Z. V.; Kimel, A. V.; Afanasiev, D.

doi:10.1103/physrevlett.133.246901

Article (Scientific journals)

Optical Excitation of Coherent THz Dynamics of the Rare-Earth Lattice through Resonant Pumping of f-f Electronic Transition in a Complex Perovskite DyFeO3

Gareev, T. T.; Sasani, Alireza; Khusyainov, D. I. et al.

2024 • In Physical Review Letters, 133 (24)

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10.1103/physrevlett.133.246901

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Keywords :

Ultrafast laser excitation,; THz Dynamics; Rare Earth Perovskite; DyFeO3

Abstract :

[en] Resonant pumping of the electronic 𝑓−𝑓 transitions in the orbital multiplet of dysprosium ions (Dy3+) in a complex perovskite DyFeO3 is shown to impulsively launch THz lattice dynamics corresponding to the 𝐵2⁢𝑔 phonon mode, which is dominanted by the motion of Dy3+ ions. The findings, supported by symmetry analysis and density-functional theory calculations, not only provide a novel route for highly selective excitation of the rare-earth crystal lattices but also establish important relationships between the symmetry of the electronic and lattice excitations in complex oxides.

Research Center/Unit :

Q-MAT - Quantum Materials - ULiège

Disciplines :

Physics

Author, co-author :

Gareev, T. T. ; Radboud University Nijmegen

Sasani, Alireza ; Université de Liège - ULiège > Département de physique > Physique théorique des matériaux ; Université de Lige

Khusyainov, D. I. ; Radboud University Nijmegen

Bousquet, Eric ; Université de Liège - ULiège > Département de physique ; Université de Lige

Gareeva, Z. V. ; Ufa Federal Research Center of the RAS ; Ufa University of Science and Technology

Kimel, A. V. ; Radboud University Nijmegen

Afanasiev, D. ; Radboud University Nijmegen

Language :

English

Title :

Optical Excitation of Coherent THz Dynamics of the Rare-Earth Lattice through Resonant Pumping of f-f Electronic Transition in a Complex Perovskite DyFeO3

Publication date :

09 December 2024

Journal title :

Physical Review Letters

ISSN :

0031-9007

eISSN :

1079-7114

Publisher :

American Physical Society (APS)

Volume :

133

Issue :

Peer reviewed :

Peer Reviewed verified by ORBi

Tags :

CÉCI : Consortium des Équipements de Calcul Intensif
Tier-1 supercomputer

Additional URL :

https://link.aps.org/article/10.1103/PhysRevLett.133.246901

European Projects :

H2020 - 861300 - COMRAD - Cold Opto-Magnetism for Random Access Devices

Funders :

EU - European Union
European Union. Marie Skłodowska-Curie Actions
ERC - European Research Council
OCW - Ministerie van Onderwijs, Cultuur en Wetenschap

Available on ORBi :

since 17 December 2024

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