[en] We have studied the formation of ultracold RbSr molecules with laser pulses. After discussing the advantages
of the Mott insulator phase for the control with pulses, we present two classes of strategies. The first class
involves two electronic states. Two extensions of stimulated Raman adiabatic passage (STIRAP) for multilevel
transitions are used: alternating STIRAP (A-STIRAP) and straddle STIRAP (S-STIRAP). Both transfer dynamics
are modeled and compared. The second class of strategies involves only the electronic ground state and uses
infrared (IR) and terahertz (THz) pulses. The molecular bond is first created by the application of a THz chirped
pulse or π-pulse. Subsequently, the molecules are transferred to their rovibrational ground level using IR pulses.
For this last step, different optimized pulse sequences that were obtained through optimal control techniques
have been studied. The relative merits of these strategies in terms of efficiency and robustness are discussed with
respect to the experimental feasibility based on present laser technologies.
Disciplines :
Physics
Author, co-author :
Devolder, Adrien
Desouter, Michèle ; Université de Liège - ULiège > Département de chimie (sciences) > Département de chimie (sciences)
Atabek, Osman
Luc-Koenig, Eliane
Dulieu, Olivier
Language :
English
Title :
Laser control of ultracold molecule formation: The case of RbSr
Publication date :
2021
Journal title :
Physical Review. A, Atomic, molecular, and optical physics
ISSN :
1050-2947
eISSN :
1094-1622
Publisher :
American Physical Society, United States - Maryland
scite shows how a scientific paper has been cited by providing the context of the citation, a classification describing whether it supports, mentions, or contrasts the cited claim, and a label indicating in which section the citation was made.
Bibliography
I. Bloch, Nature (London) 453, 1016 (2008) NATUAS 0028-0836 10.1038/nature07126.
A. Micheli, G. K. Brennen, and P. Zoller, Nat. Phys. 2, 341 (2006) 1745-2473 10.1038/nphys287.
I. M. Georgescu, S. Ashhab, and F. Nori, Rev. Mod. Phys. 86, 153 (2014) RMPHAT 0034-6861 10.1103/RevModPhys.86.153.
B. Yan, A. Moses, B. Gadway, J. P. Covey, K. R. A. Hazzard, A. M. Rey, D. S. Jin, and J. Ye, Nature (London) 501, 521 (2013) NATUAS 0028-0836 10.1038/nature12483.
R. Barnett, D. Petrov, M. Lukin, and E. Demler, Phys. Rev. Lett. 96, 190401 (2006) PRLTAO 0031-9007 10.1103/PhysRevLett.96.190401.
K. Shioya, K. Mishima, and K. Yamashita, Mol. Phys. 105, 1283 (2007) MOPHAM 0026-8976 10.1080/00268970701439573.
M. Karra, K. Sharma, B. Friedrich, S. Kals, and D. Herschbach, J. Chem. Phys. 144, 094301 (2016) JCPSA6 0021-9606 10.1063/1.4942928.
K. Sharma and B. Friedrich, New J. Phys. 17, 045017 (2015) NJOPFM 1367-2630 10.1088/1367-2630/17/4/045017.
D. DeMille, Phys. Rev. Lett. 88, 067901 (2002) PRLTAO 0031-9007 10.1103/PhysRevLett.88.067901.
S. F. Yelin, K. Kirby, and R. Côté, Phys. Rev. A 74, 050301 (R) (2006) PLRAAN 1050-2947 10.1103/PhysRevA.74.050301.
A. André, D. DeMille, J. M. Doyle, M. D. Lukin, S. E. Maxwell, P. Rabi, R. J. Schoelkopf, and P. Zoller, Nat. Phys. 2, 636 (2006) 1745-2473 10.1038/nphys386.
D. Sugny, L. Bomble, T. Ribeyre, O. Dulieu, and M. Desouter-Lecomte, Phys. Rev. A 80, 042325 (2009) PLRAAN 1050-2947 10.1103/PhysRevA.80.042325.
L. Bomble, P. Pellegrini, P. Ghesquière, and M. Desouter-Lecomte, Phys. Rev. A 82, 062323 (2010) PLRAAN 1050-2947 10.1103/PhysRevA.82.062323.
A. Jaouadi, E. Barrez, Y. Justum, and M. Desouter-Lecomte, J. Chem. Phys. 139, 014310 (2013) JCPSA6 0021-9606 10.1063/1.4812317.
J. Zhu, S. Kais, Q. Wei, D. Herschbach, and B. Friedrich, J. Chem. Phys. 138, 024104 (2013) JCPSA6 0021-9606 10.1063/1.4774058.
N. Balakrishnan, J. Chem. Phys. 145, 150901 (2016) JCPSA6 0021-9606 10.1063/1.4964096.
C. Makrides, J. Hazra, G. B. Pradhan, A. Petrov, B. K. Kendrick, T. González-Lezana, N. Balakrishnan, and S. Kotochigova, Phys. Rev. A 91, 012708 (2015) PLRAAN 1050-2947 10.1103/PhysRevA.91.012708.
E. R. Hudson, H. J. Lewandowski, B. C. Sawyer, and J. Ye, Phys. Rev. Lett. 96, 143004 (2006) PRLTAO 0031-9007 10.1103/PhysRevLett.96.143004.
S. Truppe, R. J. Hendricks, S. K. Tokunaga, H. J. Lewandowski, M. G. Kovlov, C. Henkel, E. A. Hinds, and M. R. Tarbutt, Nat. Commun. 4, 2600 (2013) 2041-1723 10.1038/ncomms3600.
J. J. Hudson, D. M. Kara, I. J. Smallman, B. E. Sauer, M. R. Tarbutt, and E. A. Hinds, Nature (London) 473, 493 (2011) NATUAS 0028-0836 10.1038/nature10104.
J. Baron, W. C. Campbell, D. DeMille, J. M. Doyle, and G. Gabrielse (ACME Collaboration), Science 343, 269 (2014) SCIEAS 0036-8075 10.1126/science.1248213.
S. K. Tokunaga, C. Stoeffer, F. Auguste, A. Shelkovnikov, C. Daussy, A. Amy-Klein, C. Chardonnet, and B. Darquié, Mol. Phys. 111, 2363 (2013) MOPHAM 0026-8976 10.1080/00268976.2013.821186.
E. A. Donley, N. R. Claussen, S. T. Thompson, and C. E. Wieman, Nature (London) 417, 529 (2002) NATUAS 0028-0836 10.1038/417529a.
E. Hodby, S. T. Thompson, C. A. Regal, M. Greiner, A. C. Wilson, D. S. Jin, E. A. Cornell, and C. E. Wieman, Phys. Rev. Lett. 94, 120402 (2005) PRLTAO 0031-9007 10.1103/PhysRevLett.94.120402.
E. Timmermans, P. Tommasini, M. Hussein, and A. Kerman, Phys. Rep. 315, 199 (1999) PRPLCM 0370-1573 10.1016/S0370-1573(99)00025-3.
C. Chin, R. Grimm, P. S. Julienne, and E. Tiesinga, Rev. Mod. Phys. 82, 1225 (2010) RMPHAT 0034-6861 10.1103/RevModPhys.82.1225.
E. Tiesinga, B. J. Verhaar, and H. T. C. Stoof, Phys. Rev. A 47, 4114 (1993) PLRAAN 1050-2947 10.1103/PhysRevA.47.4114.
K. Winkler, F. Lang, G. Thalhammer, P. van der Staten, R. Grimm, and J. Hecker Denschlag, Phys. Rev. Lett. 98, 043201 (2007) PRLTAO 0031-9007 10.1103/PhysRevLett.98.043201.
Y. Liu, T. Gong, Z. JI, G. Wang, Y. Zhao, L. Xiao, and S. Jia, J. Chem. Phys. 151, 084303 (2019) JCPSA6 0021-9606 10.1063/1.5108637.
M. Tomza, F. Pawlowski, M. Jeziorska, C. P. Koch, and R. Moszynski, Phys. Chem. Chem. Phys. 13, 18893 (2011) PPCPFQ 1463-9076 10.1039/c1cp21196j.
V. Barbé, A. Ciamei, B. Pasquiou, L. Reichsöllner, F. Schreck, P. S. Zuchowski, and J. M. Hutson, Nat. Phys. 14, 881 (2018) 1745-2473 10.1038/s41567-018-0169-x.
A. Fioretti, D. Comparat, A. Crubellier, O. Dulieu, F. Masnou-Seeuws, and P. Pillet, Phys. Rev. Lett. 80, 4402 (1998) PRLTAO 0031-9007 10.1103/PhysRevLett.80.4402.
S. Stellmer, B. Pasquiou, R. Grimm, and F. Schreck, Phys. Rev. Lett. 109, 115302 (2012) PRLTAO 0031-9007 10.1103/PhysRevLett.109.115302.
A. Ciamei, A. Bayerle, C.-C. Chen, B. Pasquiou, and F. Schreck, Phys. Rev. A 96, 013406 (2017) 2469-9926 10.1103/PhysRevA.96.013406.
V. S. Malinovsky and D. J. Tannor, Phys. Rev. A 56, 4929 (1997) PLRAAN 1050-2947 10.1103/PhysRevA.56.4929.
I. R. Solá, V. S. Malinovsky, and D. J. Tannor, Phys. Rev. A 60, 3081 (1999) PLRAAN 1050-2947 10.1103/PhysRevA.60.3081.
N. V. Vitanov, A. A. Rangelov, B. W. Shore, and K. Bergmann, Rev. Mod. Phys. 89, 015006 (2017) RMPHAT 0034-6861 10.1103/RevModPhys.89.015006.
S. Kotochigova, Phys. Rev. lett. 99, 073003 (2007) PRLTAO 0031-9007 10.1103/PhysRevLett.99.073003.
E. Juarros, P. Pellegrini, K. Kirby, and R. Coté, Phys. Rev. A 73, 041403 (R) (2006) PLRAAN 1050-2947 10.1103/PhysRevA.73.041403.
E. Luc-Koenig, R. Kosloff, F. Masnou-Seeuws, and M. Vatasescu, Phys. Rev. A 70, 033414 (2004) PLRAAN 1050-2947 10.1103/PhysRevA.70.033414.
R. Lefebvre and O. Atabek, Phys. Rev. A 101, 063406 (2020) 2469-9926 10.1103/PhysRevA.101.063406.
M. Lewenstein, A. Sanpera, and V. Ahufinger, Ultracold Atoms in Optical Lattices (Oxford University Press, Oxford, 2012).
T. Volz, N. Syassen, D. M. Bauer, E. Hansis, S. Dürr, and G. Rempe, Nat. Phys. 2, 692 (2006) 1745-2473 10.1038/nphys415.
G. Thalhammer, K. Winkler, F. Lang, S. Schmid, R. Grimm, and J. H. Denschlag, Phys. Rev. Lett. 96, 050402 (2006) PRLTAO 0031-9007 10.1103/PhysRevLett.96.050402.
B. Damski, L. Santos, E. Tiemann, M. Lewenstein, S. Kotochigova, P. Julienne, and P. Zoller, Phys. Rev. Lett. 90, 110401 (2003) PRLTAO 0031-9007 10.1103/PhysRevLett.90.110401.
T. Stöferle, H. Moritz, K. Gunter, M. Köhl, and T. Esslinger, Phys. Rev. Lett. 96, 030401 (2006) PRLTAO 0031-9007 10.1103/PhysRevLett.96.030401.
C. Ospelkaus, S. Ospelkaus, L. Humbert, P. Ernst, K. Sengstock, and K. Bongs, Phys. Rev. Lett. 97, 120402 (2006) PRLTAO 0031-9007 10.1103/PhysRevLett.97.120402.
J. K. Freericks, M. M. Maśka, A. Hu, T. M. Hanna, C. J. Williams, P. S. Julienne, and R. Lemanski, Phys. Rev. A 81, 011605 (R) (2010) PLRAAN 1050-2947 10.1103/PhysRevA.81.011605.
S. A. Moses, J. P. Covey, M. T. Miecnikowski, B. Yan, B. Gadway, J. Ye, and D. S. Jin, Science 350, 659 (2015) SCIEAS 0036-8075 10.1126/science.aac6400.
J. P. Covey, S. A. Moses, M. Gärttner, A. Safavi-Naini, M. T. Miecnikowski, Z. Fu, J. Schachenmayer, P. S. Julienne, A. M. Rey, D. S. Jin, and J. Ye, Nat. Commun. 7, 11279 (2016) 2041-1723 10.1038/ncomms11279.
L. Reichsöllner, A. Schindewolf, T. Takekoshi, R. Grimm, and H.-C. Nägerl, Phys. Rev. Lett. 118, 073201 (2017) PRLTAO 0031-9007 10.1103/PhysRevLett.118.073201.
N. V. Vitanov, T. Halfmann, B. W. Shore, and K. Bergmann, Annu. Rev. Phys. Chem. 52, 763 (2001) ARPLAP 0066-426X 10.1146/annurev.physchem.52.1.763.
L. R. Liu, J. D. Hood, Y. Yu, J. T. Zhang, N. R. Hutzler, T. Rosenband, and K. K. Ni, Science 360, 900 (2018) SCIEAS 0036-8075 10.1126/science.aar7797.
L. R. Liu, J. D. Hood, Y. Yu, J. T. Zhang, K. Wang, Y.-W. Lin, T. Rosenband, and K. K. Ni, Phys. Rev. X 9, 021039 (2019) 2160-3308 10.1103/PhysRevX.9.021039.
F. Deuretzbacher, K. Plassmeier, D. Pfannkuche, F. Werner, C. Ospelkaus, S. Ospelkaus, K. Sengstock, and K. Bongs, Phys. Rev. A 77, 032726 (2008) PLRAAN 1050-2947 10.1103/PhysRevA.77.032726.
S. Grishkevich and A. Saenz, Phys. Rev. A 76, 022704 (2007) PLRAAN 1050-2947 10.1103/PhysRevA.76.022704.
S. Grishkevich and A. Saenz, Phys. Rev. A 80, 013403 (2009) PLRAAN 1050-2947 10.1103/PhysRevA.80.013403.
S. Grishkevich, S. Sala, and A. Saenz, Phys. Rev. A 84, 062710 (2011) PLRAAN 1050-2947 10.1103/PhysRevA.84.062710.
P. S. Zuchowski, R. Guérout, and O. Dulieu, Phys. Rev. A 90, 012507 (2014) PLRAAN 1050-2947 10.1103/PhysRevA.90.012507.
A. Devolder, E. Luc-Koenig, O. Atabek, M. Desouter-Lecomte, and O. Dulieu, Phys. Rev. A 98, 053411 (2018) 2469-9926 10.1103/PhysRevA.98.053411.
V. Kokoouline, O. Dulieu, R. Kosloff, and F. Masnou-Seeuws, J. Chem. Phys. 110, 9865 (1999) JCPSA6 0021-9606 10.1063/1.478860.
K. Willner, O. Dulieu, and F. Masnou-Seeuws, J. Chem. Phys. 120, 548 (2004) JCPSA6 0021-9606 10.1063/1.1630031.
S. Kallush and R. Kosloff, Chem. Phys. Lett. 433, 221 (2006) CHPLBC 0009-2614 10.1016/j.cplett.2006.11.040.
O. A. Rubtsova, V. I. Kukulin, and V. N. Pomerantsev, Ann. Phys. 360, 613 (2015) APNYA6 0003-4916 10.1016/j.aop.2015.04.028.
O. Dulieu and P. S. Julienne, J. Chem. Phys. 103, 60 (1995) JCPSA6 0021-9606 10.1063/1.469622.
O. Dulieu, R. Kosloff, F. Masnou-Seeuws, and G. Pichler, J. Chem. Phys. 107, 10633 (1997) JCPSA6 0021-9606 10.1063/1.474179.
S. Kallush, R. Kosloff, and F. Masnou-Seeuws, Phys. Rev. A 75, 043404 (2007) PLRAAN 1050-2947 10.1103/PhysRevA.75.043404.
V. Kokoouline, O. Dulieu, R. Kosloff, and F. Masnou-Seeuws, Phys. Rev. A 62, 032716 (2000) PLRAAN 1050-2947 10.1103/PhysRevA.62.032716.
V. Kokoouline, O. Dulieu, and F. Masnou-Seeuws, Phys. Rev. A 62, 022504 (2000) PLRAAN 1050-2947 10.1103/PhysRevA.62.022504.
P. Pellegrini, O. Dulieu, and F. Masnou-Seeuws, Eur. Phys. J. D 20, 77 (2002) EPJDF6 1434-6060 10.1140/epjd/e2002-00120-5.
J. G. Danzl, M. J. Mark, E. Haller, M. Gustavsson, R. Hart, J. Aldegunde, J. M. Hutson, and H.-C. Nägerl, Nat. Phys. 6, 265 (2010) 1745-2473 10.1038/nphys1533.
E. F. de Lima, Phys. Rev. A 95, 013411 (2017) 2469-9926 10.1103/PhysRevA.95.013411.
A. Devolder, E. Luc-Koenig, O. Atabek, M. Desouter-Lecomte, and O. Dulieu, Phys. Rev. A 100, 052703 (2019) 2469-9926 10.1103/PhysRevA.100.052703.
S. Guérin, V. Hakobyan, and H. R. Jauslin, Phys. Rev. A 84, 013423 (2011) PLRAAN 1050-2947 10.1103/PhysRevA.84.013423.
V. S. Malinovsky and L. Krause, Eur. Phys. J. D 14, 147 (2001) EPJDF6 1434-6060 10.1007/s100530170212.
G. F. Thomas, Phys. Rev. A 27, 2744 (1983) 0556-2791 10.1103/PhysRevA.27.2744.
M. Holthaus and B. Just, Phys. Rev. A 49, 1950 (1994) PLRAAN 1050-2947 10.1103/PhysRevA.49.1950.
C. Brit, R. Chakrabarti, and H. Rabitz, New J. Phys 12, 075008 (2010) NJOPFM 1367-2630 10.1088/1367-2630/12/7/075008.
W. Zhu, J. Botina, and H. Rabitz, J. Chem. Phys. 108, 1953 (1998) JCPSA6 0021-9606 10.1063/1.475576.
S. Chelkowski, A. D. Bandrauk, and P. B. Corkum, Phys. Rev. Lett. 65, 2355 (1990) PRLTAO 0031-9007 10.1103/PhysRevLett.65.2355.
M. Sugawara and Y. Fujimura, J. Chem. Phys. 100, 5646 (1994) JCPSA6 0021-9606 10.1063/1.467132.
Similar publications
Sorry the service is unavailable at the moment. Please try again later.
This website uses cookies to improve user experience. Read more
Save & Close
Accept all
Decline all
Show detailsHide details
Cookie declaration
About cookies
Strictly necessary
Performance
Strictly necessary cookies allow core website functionality such as user login and account management. The website cannot be used properly without strictly necessary cookies.
This cookie is used by Cookie-Script.com service to remember visitor cookie consent preferences. It is necessary for Cookie-Script.com cookie banner to work properly.
Performance cookies are used to see how visitors use the website, eg. analytics cookies. Those cookies cannot be used to directly identify a certain visitor.
Used to store the attribution information, the referrer initially used to visit the website
Cookies are small text files that are placed on your computer by websites that you visit. Websites use cookies to help users navigate efficiently and perform certain functions. Cookies that are required for the website to operate properly are allowed to be set without your permission. All other cookies need to be approved before they can be set in the browser.
You can change your consent to cookie usage at any time on our Privacy Policy page.
