Article (Scientific journals)
Lattice dynamics and thermoelectric properties of nanocrystalline silicon-germanium alloys
Claudio, T.; Stein, N.; Petermann, N. et al.
2016In Physica Status Solidi A. Applications and Materials Science, 213 (3), p. 515-523
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Keywords :
Si-Ge alloys; BiCMOS technology; Crystal lattices; Dynamics; Germanium; Inelastic neutron scattering; Lattice vibrations; Nanocrystalline alloys; Nanocrystalline silicon; Nanocrystals; Neutron scattering; Phosphorus; Silicon alloys; Sintering; Specific heat; Temperature; Thermoelectric equipment; Low temperature heat capacities; Nanostructured silicon germaniums; Phosphorus doping; Silicon-germanium alloys; Thermoelectric properties; Thermoelectric transport; Thermoelectric transport properties; Germanium alloys
Abstract :
[en] The lattice dynamics and thermoelectric properties of sintered phosphorus-doped nanostructured silicon-germanium alloys obtained by gas-phase synthesis were studied. Measurements of the density of phonon states by inelastic neutron scattering were combined with measurements of the elastic constants and the low-temperature heat capacity. A strong influence of nanostructuring and alloying on the lattice dynamics was observed. The thermoelectric transport properties of samples with different doping as well as samples sintered at different temperature were characterized between room temperature and 1000°C. A peak figure of merit zT=0.88 at 900°C is observed and is comparatively insensitive to the aforementioned parameter variations. © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Disciplines :
Chemistry
Author, co-author :
Claudio, T.;  Jülich Centre for Neutron Science JCNS, Peter Grünberg Institut PGI, JARA-FIT, Forschungszentrum Jülich GmbH, Jülich, Germany, Faculté des Sciences, Université de Liège, Liège, Belgium
Stein, N.;  Faculty of Engineering, Center for Nano-integration Duisburg-Essen (CENIDE), University of Duisburg-Essen, Duisburg, Germany
Petermann, N.;  Faculty of Engineering, Center for Nano-integration Duisburg-Essen (CENIDE), University of Duisburg-Essen, Duisburg, Germany
Stroppa, D. G.;  Peter Grünberg Institut PGI-5, Forschungszentrum Jülich GmbH, Jülich, Germany
Koza, M. M.;  Institut Laue Langevin, 71 Avenue des Martyrs, Grenoble, France
Wiggers, H.;  Faculty of Engineering, Center for Nano-integration Duisburg-Essen (CENIDE), University of Duisburg-Essen, Duisburg, Germany
Klobes, B.;  Jülich Centre for Neutron Science JCNS, Peter Grünberg Institut PGI, JARA-FIT, Forschungszentrum Jülich GmbH, Jülich, Germany
Schierning, G.;  Faculty of Engineering, Center for Nano-integration Duisburg-Essen (CENIDE), University of Duisburg-Essen, Duisburg, Germany
Hermann, Raphaël ;  Université de Liège - ULiège > Département de chimie (sciences) > Département de chimie (sciences)
Language :
English
Title :
Lattice dynamics and thermoelectric properties of nanocrystalline silicon-germanium alloys
Publication date :
2016
Journal title :
Physica Status Solidi A. Applications and Materials Science
ISSN :
1862-6300
eISSN :
1862-6319
Publisher :
Wiley - VCH Verlag, Weinheim, Germany
Volume :
213
Issue :
3
Pages :
515-523
Peer reviewed :
Peer Reviewed verified by ORBi
Available on ORBi :
since 14 November 2020

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