Elasticity and magnetocaloric effect in MnFe4Si3

[en] The room temperature magnetocaloric material MnFe4Si3 was investigated with nuclear inelastic scattering (NIS) and resonant ultrasound spectroscopy (RUS) at different temperatures and applied magnetic fields in order to assess the influence of the magnetic transition and the magnetocaloric effect on lattice dynamics. The NIS data give access to phonons with energies above 3 meV, whereas RUS probes the elasticity of the material in the MHz frequency range and thus low-energy, ∼ neV, phonon modes. A significant influence of the magnetic transition on the lattice dynamics is observed only in the low-energy, long-wavelength limit. MnFe4Si3 and other compounds in the Mn5-xFexSi3 series were also investigated with vibrating sample magnetometry, resistivity measurements, and Mössbauer spectroscopy in order to study the magnetic transitions and to complement the results obtained on the lattice dynamics. © 2016 American Physical Society.

Disciplines :

Chemistry

Author, co-author :

Herlitschke, Marcus ; FS-PE, Deutsches Elektronen-Synchrotron (DESY), Hamburg, Germany, Jülich Centre for Neutron Science JCNS, Peter Grünberg Institut PGI, JARA-FIT, Forschungszentrum Jülich GmbH, Jülich, Germany, Faculté des Sciences, Université de Liège, Liège, Belgium

Klobes, B.; Jülich Centre for Neutron Science JCNS, Peter Grünberg Institut PGI, JARA-FIT, Forschungszentrum Jülich GmbH, Jülich, Germany

Sergueev, I.; FS-PE, Deutsches Elektronen-Synchrotron (DESY), Hamburg, Germany

Hering, P.; Jülich Centre for Neutron Science JCNS, Peter Grünberg Institut PGI, JARA-FIT, Forschungszentrum Jülich GmbH, Jülich, Germany

Perßon, J.; Jülich Centre for Neutron Science JCNS, Peter Grünberg Institut PGI, JARA-FIT, Forschungszentrum Jülich GmbH, Jülich, Germany

Hermann, Raphaël ; Université de Liège - ULiège > Département de chimie (sciences) > Département de chimie (sciences)

Language :

English

Title :

Elasticity and magnetocaloric effect in MnFe4Si3

Publication date :

2016

Journal title :

Physical Review. B

ISSN :

2469-9950

eISSN :

2469-9969

Publisher :

American Physical Society

Volume :

Issue :

Pages :

094304

Peer reviewed :

Peer Reviewed verified by ORBi

Name of the research project :

VH NG-407 “Lattice dynamics in emerging functional materials”

Funders :

HGF - Helmholtz-Gemeinschaft Deutscher Forschungszentren [DE]
DOE - United States. Department of Energy [US-OR]

Available on ORBi :

since 11 November 2020

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