Ni-substitution effect on the properties of Ba0.5Sr1.5Zn2-xNixFe12O22 powders

Magnetic phase transitions; Magnetic properties; Ni-substitution; Sol–gel auto-combustion; Y-type hexaferrites; Barium compounds; Combustion; Iron compounds; Magnetic materials; Magnetic susceptibility; Magnetization; Powders; Sols; Strontium compounds; Zinc compounds; Ac susceptibility; Auto combustion; Auto-combustion methods; Ferromagnetic state; Hexa-ferrites; Magnetization values; Structural and magnetic properties; Nickel compounds

Abstract :

[en] We consider the influence of the magnetic cation (Ni2+) substitution on the structural and magnetic properties of Ba0.5Sr1.5Zn2-xNixFe12O22 (x = 0.8, 1, 1.5) powders. The powders were synthesized by using the citric-acid sol–gel auto-combustion method. Their ac-magnetization was measured in an ac-magnetic field with an amplitude of 10 Oe and a frequency of 1000 Hz to detect any magnetic phase transitions. A strong influence of the Ni-substitution on the magnetic properties was thus observed. A magnetic phase transition from a helicoidal to a ferrimagnetic spin order at 284 K was observed for the sample Ba0.5Sr1.5Zn0.5Ni1.5Fe12O22. The magnetic-phase transition from conical spin order to hellicoidal spin order was registered at 149 K and 177 K for x = 0.8 and x = 1, respectively. Triple hysteresis loops were observed for all samples at 4.2 K, which indicates the presence of two kinds of ferromagnetic states with different magnetization values. © 2020 Elsevier B.V.

Disciplines :

Chemistry
Physics

Author, co-author :

Koutzarova, T.; Institute of Electronics, Bulgarian Academy of Sciences, 72 Tsarigradsko Chaussee, Sofia, 1784, Bulgaria

Kolev, S.; Institute of Electronics, Bulgarian Academy of Sciences, 72 Tsarigradsko Chaussee, Sofia, 1784, Bulgaria

Krezhov, K.; Institute of Electronics, Bulgarian Academy of Sciences, 72 Tsarigradsko Chaussee, Sofia, 1784, Bulgaria

Georgieva, B.; Institute of Electronics, Bulgarian Academy of Sciences, 72 Tsarigradsko Chaussee, Sofia, 1784, Bulgaria

Ghelev, C.; Institute of Electronics, Bulgarian Academy of Sciences, 72 Tsarigradsko Chaussee, Sofia, 1784, Bulgaria

Kovacheva, D.; Institute of General and Inorganic Chemistry, Bulgarian Academy of Sciences, Acad. Georgi Bonchev Str., bld. 11, Sofia, 1113, Bulgaria

Vertruyen, Bénédicte ; Université de Liège - ULiège > Département de chimie (sciences) > Chimie inorganique structurale

Closset, Raphaël ; Université de Liège - ULiège > Département de chimie (sciences) > Département de chimie (sciences)

Tran, L. M.; Institute of Low Temperature and Structure Research, Polish Academy of Sciences, Ul. Okólna 2, Wroclaw, 50-422, Poland

Babij, M.; Institute of Low Temperature and Structure Research, Polish Academy of Sciences, Ul. Okólna 2, Wroclaw, 50-422, Poland

Zaleski, A. J.; Institute of Low Temperature and Structure Research, Polish Academy of Sciences, Ul. Okólna 2, Wroclaw, 50-422, Poland

Language :

English

Title :

Ni-substitution effect on the properties of Ba0.5Sr1.5Zn2-xNixFe12O22 powders

Publication date :

2020

Journal title :

Journal of Magnetism and Magnetic Materials

ISSN :

0304-8853

eISSN :

1873-4766

Publisher :

Elsevier B.V.

Volume :

505

Pages :

166725

Peer reviewed :

Peer Reviewed verified by ORBi

Additional URL :

https://doi.org/10.1016/j.jmmm.2020.166725

Funders :

BAS - Bulgarian Academy of Sciences [BG]
PAN - Polska Akademia Nauk [PL]
WBI - Wallonie-Bruxelles International [BE]

Available on ORBi :

since 13 July 2020

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