[en] Ruthenium-N-heterocyclic carbene complexes with the generic formula [RuHCl(CO)(NHC)(PCy3)] exhibit a high catalytic activity toward the (E)-selective silylative coupling of divinyl-substituted double-decker silsesquioxanes with two distinctly substituted styrenes. This process leads to a novel class of unsymmetrically functionalized silsesquioxane derivatives.
Disciplines :
Chemistry
Author, co-author :
Zak, Patrycja; Department of Organometallic Chemistry, Faculty of Chemistry, Adam Mickiewicz University in Poznan, Umultowska 89B, Poznan, Poland
Delaude, Lionel ; Université de Liège - ULiège > Département de chimie (sciences) > Chimie organométallique et catalyse homogène
Dudziec, Beata; Department of Organometallic Chemistry, Faculty of Chemistry, Adam Mickiewicz University in Poznan, Umultowska 89B, Poznan, Poland, Centre for Advanced Technologies, Adam Mickiewicz University in Poznan, Umultowska 89C, Poznan, Poland
Marciniec, Bogdan; Department of Organometallic Chemistry, Faculty of Chemistry, Adam Mickiewicz University in Poznan, Umultowska 89B, Poznan, Poland, Centre for Advanced Technologies, Adam Mickiewicz University in Poznan, Umultowska 89C, Poznan, Poland
Language :
English
Title :
N-Heterocyclic carbene-based ruthenium-hydride catalysts for the synthesis of unsymmetrically functionalized double-decker silsesquioxanes
Publication date :
2018
Journal title :
Chemical Communications
ISSN :
1359-7345
eISSN :
1364-548X
Publisher :
Royal Society of Chemistry, Cambridge, United Kingdom
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