[en] In this paper, structural, magnetic, and magnetocaloric properties of zinc-doped nickel ferrite,
Zn1−xNixFe2O4 (x = 0.3 and 0.4) were investigated. The samples were prepared using solid-state reaction. X-ray diffraction (XRD) and magnetization measurements were
performed to study crystallographic structure and magnetic properties. For a magnetic field changing from 0 to 5 T, the corresponding isothermal entropy change was found to be near 1.4 J/kg K for both samples. The decreasing of Ni content from x = 0.4 to 0.3, enables to shift the Curie temperature of Zn1−xNixFe2O4 from 450 K toward (325 K). As main results, it was found that the relative cooling power (RCP) could be significantly enhanced by changing
Ni concentration in Zn1−xNixFe2O4 (505 J/kg (for x = 0.3) and 670 J/kg (for x = 0.4)), which is considered as a recommended parameter for a wide temperature range in magnetic refrigeration application. Our finding should inspire and open new ways for the enhancement of the magnetocaloric effect in spinel ferrite-based materials.
Disciplines :
Chemistry
Author, co-author :
El Maalam, Khadija
Fkhar, lahcen
Mohammed, Hamedoun
Mahmoud, Abdelfattah ; Université de Liège > Département de chimie (sciences) > LCIS - GreenMAT
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