[en] The constraint of time-integrated zero area on the laser field is a fundamental requirement, both theoretically
and experimentally, in the control of molecular dynamics. By using techniques of local and optimal control theory,
we show how to enforce this constraint in two benchmark control problems, namely, molecular orientation and
photofragmentation. The origin and the physical implications for the dynamics of this zero-area control field are
discussed.
Disciplines :
Physics Chemistry
Author, co-author :
Sugny, Dominique; Université de Bourgogne > Institut Carnot
Vranckx, Stéphane; Université Libre de Bruxelles - ULB > Service de Chimie Quantique et de Photochimie
Ndong, Mamadou; Université de Bourgogne > Institut Carnot
Vaeck, Nathalie; Université Libre de Bruxelles - ULB > Service de Chimie Quantique et de Photophysique
Atabek, Osman; Université Paris-Sud 11 > Institut des Sciences Moléculaires ISMO
Desouter-Lecomte, Michèle ; Université de Liège - ULiège > Département de chimie (sciences) > Département de chimie (sciences)
Language :
English
Title :
Control of molecular dynamics with zero-area fields. application to molecular orientation and photodissociation
Publication date :
November 2014
Journal title :
Physical Review. A, Atomic, molecular, and optical physics
ISSN :
1050-2947
eISSN :
1094-1622
Publisher :
American Physical Society, United States - Maryland
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